Low-Loss Dielectric Nanoantennas for Surface-Enhanced Fluorescence Spectroscopy and Nonlinear Photonics

G. GRINBLAT; Y. LI; J. CAMBIASSO; T. SHIBANUMA; M. P. NIELSEN; E. CORTÉS; P. ALBELLA; A. RAKOVICH; R. F. OULTON; S. A. MAIER

Conferencia; The 9th International Conference on Materials for Advanced Technologies; 2017

Dielectric nanoantennas have recently emerged as promising alternative candidates to plasmonic systems in the visible range.[1,2] When excited above their bandgap energies, high-refractive-index dielectric nanostructures can highly concentrate electric and magnetic fields within subwavelength volumes while presenting ultra-low absorption compared to metals.[3] In particular, by locally enhancing the incident light intensity, dielectric nanoantennas are expected not only to produce negligible heating, but also boost nonlinear phenomena and surface-enhanced spectroscopies, since their efficiencies increase with the excitation density.In this presentation, GaP and Ge nanoantennas will be introduced as promising nanosystems for surface-enhanced fluorescence and second and third harmonic generation on the nanoscale at visible wavelengths.[3-5] In addition, hybrid dielectric/metallic Si/Au nanoantennas will also be analyzed.[6] Fluorescence enhancement factors of over 3000 and harmonic conversion efficiencies on the order of 1E-3% will be demonstrated for this suitably engineered dielectric-based nanostructures. [1] Albella, P.; Poyli, M. A.; Schmidt, M. K.; Maier, S. A.; Moreno, F.; Sáenz, J. J.; Aizpurua, J. J. Phys. Chem. C 2013, 117, 13573-13584.[2] Shorokhov, A. S.; Melik-Gaykazyan, E. V.; Smirnova, D. A.; Hopkins, B.; Chong, K. E.; Choi, D. Y.; Shcherbakov, M. R.; Miroshnichenko, A. E.; Neshev, D. N.; Fedyanin, A. A.; Kivshar, Y. S. Nano Lett. 2016, 16, 4857-4861.[3] Grinblat, G.; Li, Y.; Nielsen, M., Oulton R. F.; Maier S. A. Nano Lett. 2016, 16, 4635-4640.[4] Grinblat, G.; Li, Y.; Nielsen, M., Oulton R. F.; Maier S. A. ACS Nano 2017, 11, 953-960.[5] Cambiasso, J.; Grinblat, G.; Li, Yi.; Rakovich, A.; Cortés, E.; Maier, S. A. Nano Lett. 2017, 17, 1219-1225.[6] Shibanuma, T.; Grinblat, G.; Albella, P.; Maier S. A. Nano Lett. 2017, 17, 2647-2651.