Time-dependent theory of reconstruction of attosecond harmonic beating by interference of multiphoton transitions

LÓPEZ, SEBASTIÁN D.; OCELLO, MATÍAS L.; ARBÓ, DIEGO G.

Physical Review A

American Physical Society

Lugar: New York; Año: 2024 vol. 110

2469-9926

Phase and time delays of atomic above-threshold ionization are usually experimentally explored by the reconstruction of attosecond harmonic beating by interference of two-photon transitions (RABBIT) technique. Theoretical studies of RABBIT rely on the perturbative treatment of the probe (near infrared or visible) laser pulse with respect to the atomic electric field and the pump composed of a train of attosecond pulses made of several harmonics with frequencies multiple of the probe fundamental frequency. In this work we present a semiclassical nonperturbative description of the phase delays for the emission of electrons from hydrogen atoms based on the strong-field approximation as the relative phase between pump and probe pulses is varied, where more than two photons are involved. Ionization times are calculated within the saddle-point approximations and serve to individualize the different electron wave packets that produce the RABBIT-like interferometric scheme. We observe different behaviors of the phase delays at different intensities of the probe. For example, for moderate and intense probe fields, the harmonics and sidebands happen to be in phase (≳4×1011W/cm2). In turn, when the probe field is sufficiently weak, we recover the well-known rule of thumb for the phase delays developed within the perturbative RABBIT theory [see D. Guénot et al., Phys. Rev. A 85, 053424 (2012)]. We show that the intracycle interference of the different paths contributing to the final energy (sideband or high harmonic) is responsible for the different behaviors of the interference pattern. Comparisons with the numerical solution of the strong-field approximation and time-dependent Schrödinger equation confirm the reliability of our semiclassical nonperturbative theory.