Modeling and experimental validation of a membrane reactor for WGSR

CAROLINA A. CORNAGLIA; MARÍA E. ADROVER; JOHN F. MÚNERA; MARISA N. PEDERNERA; EDUARDO A. LOMBARDO; DANIEL O. BORIO

Maastrich

Simposio; International Symposium on Chemical Reaction Engineering (ISCRE 22); 2012

A heterogeneous 1D model was used to represent the behavior of a membrane reactor forWGSR. The model was validated with experimental data, obtained from a laboratory scalemembrane reactor. Experiments were carried out under isothermal conditions using a Pt(0.6)/La2O3.SiO2 catalyst. The effect of the sweep gas flow rate on the CO conversion and H2recovery was analyzed. Hydrogen partial-pressure axial profiles were included to justify themodel selection. The influence of other operating variables (space velocity, temperature) wasalso addressed.